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    The He2 - OCS Complex: Comparison Between Theory and Experiment

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    Carrington_et_al_2017 _ju The_He2_-_OCS_complex_comparison_between_theory_an.pdf (370.6Kb)
    Date
    2017-10-31
    Author
    Oliaee, J. Norooz
    Moazzen-Ahmadi, N.
    McKellar, A.R.W.
    Wang, Xiao-Gang
    Carrington, Tucker Jr
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    Abstract
    OCS is an ideal probe for quantum solvation effects in cold helium clusters. He2-OCS is the “second step” in going from a single OCS molecule to a large doped superfluid helium cluster. Here assignment of the spectrum of He2-OCS is significantly extended to higher values of J, K, and vt (the low frequency torsional vibration). The observation of a new infrared band, OCS n1 + n3, taken together with the known n1 band, enables assignments to be verified by comparing ground state combination differences. Relatively straightforward scaling of

    previously calculated theoretical energy levels gives a remarkably good fit to experiment.
    URI for this record
    http://hdl.handle.net/1974/23829
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