Distributed Generation Reformer and Fuel Cell System Modeling and Reformer Catalyst Layer Optimization

dc.contributor.authorDePippo, Kurtisen
dc.contributor.departmentChemical Engineeringen
dc.contributor.supervisorPeppley, Brant A.en
dc.date2016-11-01 15:09:14.063
dc.degree.grantorQueen's University at Kingstonen
dc.descriptionThesis (Master, Chemical Engineering) -- Queen's University, 2016-11-01 15:09:14.063en
dc.description.abstractThis research presents a diesel-fed steam reformer and solid oxide fuel cell stack system Honeywell UniSim® Design Suites model and a two-dimensional diesel-fed steam reformer ANSYS Fluent model. The performance of the reformer and fuel cell system was compared to the performance of diesel generators in Canadian remote communities to illustrate the environmental and economic advantages that reformer and fuel cell systems have over typical diesel generation setups. The results show that, despite current solid oxide fuel cell technology being economically unfeasible, technology that is nearing commercialization could present substantial environmental and economic savings opportunities for diesel-based distributed generation projects. The UniSim® model relied on several assumptions, one of which was the full conversion of the fuel feed within the steam reformer. A two-dimensional steam reformer model was therefore created in ANSYS Fluent to more accurately model the reforming process. Parameter studies on the reformer catalyst layer showed that reducing catalyst layer porosity along the length of the reformer results in improved reformer performance because of increased catalyst mass and higher reaction rates downstream that help push the reforming reaction towards equilibrium.en
dc.relation.ispartofseriesCanadian thesesen
dc.rightsQueen's University's Thesis/Dissertation Non-Exclusive License for Deposit to QSpace and Library and Archives Canadaen
dc.rightsProQuest PhD and Master's Theses International Dissemination Agreementen
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dc.rightsThis publication is made available by the authority of the copyright owner solely for the purpose of private study and research and may not be copied or reproduced except as permitted by the copyright laws without written authority from the copyright owner.en
dc.subjectDiesel Reformingen
dc.subjectSteam Reformingen
dc.subjectPorous Catalyst Layer Modelingen
dc.subjectDistributed Generationen
dc.subjectReformer and Fuel Cell Systemen
dc.titleDistributed Generation Reformer and Fuel Cell System Modeling and Reformer Catalyst Layer Optimizationen
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